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You can't just copy the Windows ISO onto the USB and boot from it. you need to use software to make a bootable version. I use an old windows 7 USB boot tool that works with 10 too.

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You need to use a third party utility to make the USB drive bootable.

 

I've been using Win32 Disk Imager for when I have to make bootable drives, you might have to find something else since you're on a Mac.

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