Lagging Stream from NAS
VLC just doesn't do well streaming directly over the network. It has to do with the way it loads / buffers.
As a per device alternative to VLC, look into Kodi.
Jellyfin does not have a PS5 app. There is a Samsung TV app, but it has to be sideloaded.
For an alternative to Plex or Jellyfin you could try Emby. It has apps for both of those and more.
You do need a paid license to use many features but it is far less expensive than Plex and has better privacy options.
As far as Jellyfin not finding everything. Make sure your files are named and organized in line with the Jellyfin documentation and are in a compatible format.
Also make sure that Jellyfin has the correct permissions to access the files and write metadata near them.

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